Peter B. Catrysse, Ph.D. - Research Website

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Confinement and field concentration in phonon-polaritonic films (mid-IR)

My research on phonon-polaritonic materials involves the exploration of sub-wavelength modes at mid-infrared wavelengths (~10 μm), where there is no strong plasmonic response from either metals or semiconductors. Yet, enhancing transmission in this wavelength range is still very important. It is known as the biological finger-print regime because many organic molecules exhibit distinctive vibrational resonances in this range. Efficient detection of molecular "finger prints" is important for a wide range of spectroscopic applications.

Figure: Transmission at normal incidence through a silicon carbide (SiC) film with a two-dimensional periodic arrangement of subwavelength cylindrical holes (solid green curve). The inset shows the geometry with radius r0=2.8 μm, period a=10.4 μm, and thickness h=4 μm. The dashed gray curve is the transmission spectrum of a homogeneous SiC film. The polariton gap is represented by clear region between the gray regions. The surface resonance is indicated by the red vertical arrow. The blue horizontal arrow shows the range of the propagating mode in the hole.

In my research on phonon-polaritonic materials, I investigate the confinement and concentration of mid-infrared radiation in subwavelength holes. As an example, I numerically and experimentally demonstrate extra-ordinary transmission through subwavelength hole arrays in silicon carbide (SiC). Many molecules have unique spectral signatures in the mid-infrared. Field concentration, associated with enhanced transmission through subwavelength holes in an otherwise opaque medium, can be very beneficial for infrared spectroscopic studies where highly localized fields are required in the vicinity of the film to achieve the required sensitivity to detect trace elements.

Featured publications:

  • J Provine, P. B. Catrysse, C. Roper, R. Maboudian, S. Fan, and R. T. Howe, "Phonon polariton reflectance spectra in a silicon carbide membrane hole array," IEEE/LEOS Lasers and Electro-Optics Society Annual Meeting '07, 466, 2007.
  • J Provine, P. B. Catrysse, C. Roper, R. Maboudian, S. Fan, and R. T. Howe, "Extraordinary Transmission Through A Poly-SiC Membrane with Subwavelength Hole Arrays," IEEE/LEOS International Conference on Optical MEMS and Nanophotonics '07, 157, 2007.
  • (ISI Cited 18 times) P. B. Catrysse and S. Fan, "Near-complete transmission through subwavelength hole arrays in phonon-polaritonic thin films," Phys. Rev. B 75, 075422, 2007.[pdf]
    (Selected for Virtual Journal of Nanoscale Science and Technology 15, Issue 11, 2007)

Press coverage:

  • School of Engineering website publishes Squeezing light into small spaces a feat of physics to highlight my theoretical work and experimental collaboration in the mid-IR as part of Stanford's strategic priority in Nanoscience and Nanotechnology (2008)
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